You need to know some quantum mechanics at the level defined by the problems below.
There are many excellent books on quantum mechanics but the most suitable is Atkins: Quantum Mechanics, Chapters 1-3. You should try to understand these three chapters or their equivalent but, even if you cannot totally understand the concepts and some of the mathematics clearly, make sure that you can do the necessary manipulations.
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1. (a) State the Schrödinger equation for a one-dimensional quantum particle of mass .
(b) What is Born's interpretation of the wavefunction , and what conditions must satisfy to be physically acceptable?
(c) A particle is subject to the potential with
(i) Sketch the potential.
(ii) Show that the wavefunction satisfies the Schrödinger equation with energy provided and
The constants and need not be determined.
(iii) Explain why is not physically acceptable unless exp(
(iv) Provide an argument to show that for the region is classically forbidden.
(v) Show that the probability that the particle is found in the classically forbidden region is and that the expectation value of the kinetic energy is . You may assume that has been chosen so that is normalized.
2. (a) Show by direct substitution that the function,
where , and are constants, is a solution of the Schrodinger equation
for a particle of mass in one dimensional free space for which the potential, , is zero everywhere.
Obtain the energy, , in terms of and .
(b) Consider a particle in a one dimensional box of length , where for and and for
(i) What value must the wave-function adopt at and
(ii) Show that the condition can be satisfied at by the function in part (a).
(c) Sketch the probability distributions for a particle in the four lowest energy levels in the box described in part (b). How do these compare with the probability distribution of a classical particle in a box?
(d) For a particle of mass moving in a square two dimensional box of side , the energy levels are given by the expression
where and are two independent quantum numbers taking on the values 1, 2, 3,... By referring to this example, explain the meaning of degeneracy, as used in quantum mechanics, and deduce which of the six lowest energy levels in this problem exhibit degeneracy.
(a) Sketch (i) the radial wavefunctions and (ii) the radial distribution functions for an electron in the 1s, 2s and 2p orbitals of the hydrogen atom.
(b) The normalised wave-function for an electron in the 1s orbital of the H atom is
where is the electron-nucleus separation and is a constant.
(i) Write down an expression for the radial distribution function describing the probability of finding an electron between and
(ii) Using your answer to part (i), calculate the most probable electron-nucleus separation in terms of .
(iii) By calculating the expectation value determine the mean distance of the electron from the nucleus in terms of .
4. (a) What is meant by the Born interpretation of a quantum mechanical wave-function? Describe how the Born interpretation leads to the imposition of boundary conditions for the wave-function of a particle confined to motion on a ring.
(b) The potential energy, , for a harmonic oscillator is given by
where is the force constant and is the displacement from equilibrium. Show by direct substitution that the wave-function
where is a solution of the Schrodinger equation for a harmonic oscillator of mass . Determine the corresponding energy, expressing your answer in terms of the vibrational frequency,
(c) Determine the position of maximum probability density for this wave-function. How does the result compare (qualitatively) with the time averaged probability of finding a particle at a specific location in a classical harmonic oscillator?
(d) Assuming the harmonic oscillator is a reasonable description of the vibration of a diatomic molecule, explain briefly why
(i) D has a lower zero point energy than H.
(ii) N has a higher vibrational frequency than O.
The normalized wave-function for an electron confined to a 1-dimensional box, with infinitely high walls, is
in which is the length of the box, the position along the box, and an integer. The Schrodinger wave equation in one dimension is
(a) Sketch the appearance of for and for
(b) A simple model of the electrons in a conjugated molecule treats them as being confined to a 1-dimensional box.
(i) Estimate a value for the length of the box from the geometry of butadiene.
(ii) Use the Pauli exclusion principle to give the occupancy of the orbitals.
(iii) Calculate the lowest energy transition that can take place among electrons confined to the conjugated system of butadiene.
(iv) The walls of the box in butadiene are not infinitely high. How would a typical wave-function be modified if walls of infinite height were replaced by walls of finite height?
(v) Calculate the probability of finding an electron in the orbital within 0.1 nm of the left hand wall of the box with infinitely high walls.